23. The Postal Service, "Such Great Heights" (2003)

With its irresistible keyboard blips and ambient synth lines, "Such Great Heights" will probably stick to your ribs before frontman Ben Gibbard even begins to sing. But the lyrics are great too, especially if you're still secretly waiting for a kiss that feels "perfectly aligned." β€” C.M.

Edward Sharpe and the Magnetic Zeros, "Home" (2009)
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